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In the “S 4 Mechanism” interpretation, formation of a high oxidation state metal oxo intermediate is invoked in the S 3 → S 4 step either as low-spin Mn V =O or a high-spin oxyl, Mn IV -O · , which is sufficiently electrophilic to forge an O-O bond followed by O 2 release

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[DOI] [PMC free article] [PubMed] [Google Scholar] 29.Meier JJ, Gallwitz B, Salmen S, Goetze O, Holst JJ, Schmidt WE, Nauck MA